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Research Inventy: International Journal Of Engineering And Science
Vol.2, Issue 8 (March 2013), Pp 18-22
Issn(e): 2278-4721, Issn(p):2319-6483, Www.Researchinventy.Com
18
Characterization of Polymeric Membranes under Large
Deformations by a Neural Model
Farid Hicham1,2
, El Ghorba Mohamed1
, Erchiqui Fouad2
, M’hamed Chergui1
1
Laboratoire de Contrôle et Caractérisation Mécanique des Matériaux et des Structures
ENSEM, B.P 8118, Oasis-Route El Jadida
Casablanca, Maroc
2
Laboratoire de Bioplasturgie et Nanotechnologie, UQAT, 445, boul. de l’Université,
Rouyn-Noranda (QC), Canada J9X 5E4
Abstract: Recent progress in polymers modeling shows a need for a precise description of the material
behavior under the combined effect of the applied efforts and temperature.The Artificial Neural Networks
(ANN), whose operation is based on some properties of biological neurons, contain various architectures
strongly interrelated treating elements and offering an alternative to conventional computational approaches.
They respond in parallel to a set of inputs, and are affected by transformations more than by algorithms and
procedures. They can achieve complicated operations of Input-Output without explicit relationships (linear and
nonlinear) between all the presented data during a learning process.In our work, we are interested by the
characterization of circular thermoplastic membranes, ABS (Acrylonitrile butadiene styrene), under biaxial
deformation using the free blowing technique. Hyperelastic Mooney-Rivlin model is considered. A neural
algorithm (based on artificial neural networks) is used to model the behavior of blowing these membranes, the
results are compared with experimental studies and numerical finite differences model.
Key words : membrane, Artificial Neural Networks, free blowing, hyperelasticity, ABS.
I. INTRODUCTION
Working a polymeric sheet attached by its contour in a 3D shape is the main feature of the process of
blow molding. Generally, the deformation is very fast, non-uniform, multiaxial, and occurs at a forming
temperature above the glass transition temperature [1]. The modeling of this phenomenon remains delicate and
creates several difficulties as in the experimentation level [2] as in the modeling level in terms of important
computational time, as well as the implementation of nonlinear constitutive laws...
Often, as the bubble size increases and the internal pressure approach a maximum value beyond it there
no solution, the numerical scheme diverges. So, to remedy this problem, we consider in this work, an approach
based on an artificial neural networks model [3], to model the behavior of thermoplastic membranes.
Recently, neural networks are used in many areas include the classification, pattern recognition, speech
synthesis, diagnosis, identification and control of dynamic systems, or even to improve the quality of produced
parts in various industrial processes such as injection molding or blow molding. The use of neural networks in
the identification processes is justified by the fact that they can be well approximated nonlinear functions
through their capacity to reproduce rather complex behavior, and their performances are improving so
continuously while relying on a dynamic learning [4], which provides a robust neuronal identification vis-à-vis
the parametric variations and disturbances that can affect the operation of the system studied. Modeling using
neural networks requires among a model selection which is a crucial step in designing a neural network, as with
any non-linear model. Indeed, this phase should lead to choose the model that has a complexity that is both
sufficient to fit the data and not excessive.In this work, the power of neural networks is used to model the
nonlinear behavior in free bowing of a polymeric membrane in ABS. A multilayer neural network is used for
this application, in order to reproduce the behavior of this membrane; the results are compared with
experimentation as well as with finite difference model [5].
II. ARTIFICIAL NEURAL NETWORKS
2.1 Introduction
Neural networks have been studied since the 40's with the notion of formal neuron of McCulloch and
Pitts [6] who first developed a mathematical model of biological neuron.Hence a neural network is a
mathematical model of treatment consists of several basic interconnected neurons via weights that play the role
Characterization Of Polymeric Membranes Under Large…
19
of synapses. These weights assume values that define the behavior of the whole structure. The adaptation of the
latter through a suitable learning algorithm, allows the network to learn, memorize and generalize information.
2.2 Multilayer network
2.2 Architecture
In general, a multilayer network is composed of an input layer, an output layer, and a number of hidden
layers. Each neuron is connected to all neurons of the next layer via connections whose weights are real.
Usually, the neuron used in the hidden layers or in the output layer, performs a weighted summation of its inputs
and a nonlinear transformation which is often the sigmoid function. While the neuron used in the input layer,
simply passes its input to output.
The architecture of a multilayer network can be given by the following figure, Fig 1 :
Figure 1. Architecture of a multilayer perceptron
2.3 Learning process
The learning of a neural network means that it changes its behavior to allow it to move towards a
clearly defined purpose. In other words, learning is adjusting the connection weights so that the outputs of the
network are as close as possible to the desired outputs for all the used examples.Initially, the learning of
multilayer networks was determined by the gradient method. Then, all optimization methods have been applied
to this problem as the conjugate gradient method, the Levenberg-Marquardt [7,8]or Kalman filters… Thus,
the literature on learning of multilayer neural networks is very rich. However, we limit the study of the back-
propagation algorithm combined with a Levenberg-Marquardt optimization algorithm, which is a modified
version of the gradient method and remains the most used and most responded. This is an optimization
algorithm that seeks to minimize a cost function which covers the gap between the desired output and that
delivered by the network, to expand more knowledge, we bring the reader to references [4] and [9].
The back-propagation algorithm can be described using the following two phases:Propagation phase or
relaxation: initially, the input values are provided to the network’s input layer, then the network propagates the
information from one layer to another to the output layer, and which gives the response of network.
Back-propagation phase: that is to calculate the difference between the outputs of the network and the desired
resulting changes in weight of the output neurons. Then, retro-propagating the error to the input layer which
allows the adaptation of the weights of the hidden layer.
In our network, we used a learning algorithm by back-propagation associated with a Levenberg-Marquardt
optimization algorithm [9], with a transfer function of sigmoid type.
In our architecture, the error in the presentation of an example, denoted by E, can be given by the following
expression:
(1)
wherein, represents the component of the desired output vector. The overall error to minimize is the
sum of all errors on the database. The inputs and outputs of the neurons j and k explicit from the following
expressions:
(2)
Characterization Of Polymeric Membranes Under Large…
20
(3)
Where f is the sigmoid activation function defined by:
(4)
The adjustment of the weights of the network by the back-propagation algorithm is ensured through the
following iterative equation:
(5)
With ε and i denote the pitch and the iteration number.
The derivative of E with the weight depends on its position, in fact:
If the weight connects the hidden layer to the output layer, so:
(6)
If the weight connects the input layer to the hidden layer, then:
(7)
It should be emphasized that the convergence of the back-propagation algorithm depends on a variety of
parameters, namely:
The complexity of the database and the order of presentation of examples. Indeed, various studies have
shown that a random sample presentation allows faster learning,The structure of the neural network considered
and especially the number of neurons in the hidden layer which must not be very important to ensure the
generalization ability of the network, or very small for the network to learn,The initial setting of the algorithm
parameters, essentially the initial values of weight and iteration pitch must be chosen in a manner allowing to
have a fast convergence.
The multilayer neural network that we propose has the following structure:
Figure 2. Structure of the used multilayer neural network
The used network consists of an input layer, hidden layers, and an output layer. The number of neurons
in the output layer depends on the response contemplated by the network. For the identification program, two
neurons are required in the output layer to give the response of the excitation, while the input of the network is
the variance of the corresponding pressures. As for modeling behavior of the membrane, the neuron will output
variance in response to pressure, while the input will be presented by the stretch ratios.The experimental data are
used for network learning, also, the back-propagation algorithm is used for error of perceptron learning. Thus,
the optimization algorithm of Levenberg-Marquardt is used also in view of minimizing the error during the
operation of back propagation, this optimization technique is more powerful than other optimization algorithms,
but it requires more memory.
Inputlayercontainingan
excitationvector
Multilayer
neural
networks
Outputlayercontaininga
responsevector
Characterization Of Polymeric Membranes Under Large…
21
III. EXPERIMENTAL
The materials considered in this work is the ABS (Acrylonitrile butadiene styrene). The initial sheet
thickness was 0.46mm. The exposed circular domain of radius R=3.175 cm is heated to the softening point
inside a heating chamber using infrared heaters. When the temperature was quite uniform over the flat sheet, the
inflation was started using compressed air at a controlled flow rate. In most inflation tests the experiment ended
when the bubble burst. The bubble pressure, its height at the pole and time are recorded simultaneously using a
video camera and a data acquisition system.
IV. RESULTS
Fig 3 below shows a comparison between our neural model, finite difference model using a hyperelastic Ogden
model [10, 11], and experimental measurements.
Figure 3. Internal pressure versus the bubble height, comparison between experimental results, finite difference
model, and neural networks model
Note that the neural model we propose reproduces faithfully the behavior of the ABS membrane as
well as the finite difference model. The margin of error between the neural model and the experimental curve
remains negligible, and can also be minimized while depending on the choice of the number of hidden layers in
the network and the chosen optimization algorithm. By increasing the number of hidden layers in the network,
while keeping the same transfer function and the same optimization algorithm of Levenberg-Marquardt, the
neuronal model can be adjusted for more fitting with the experimental results,
Fig 4 below shows the results of model fitting:
Figure 4. Internal pressure versus the bubble height, comparison between experimental results, finite difference
model, and neural networks model (Adjusted model)
It is clear that the neural model that we propose reproduces the behavior of the membrane, but, the
fitting procedure that contains a number of algorithms, affects the computation time which becomes increasingly
important also with increasing the number of hidden layers in the network, which induces the addition of other
conditions nonlinearity.
Characterization Of Polymeric Membranes Under Large…
22
V. CONCLUSION
The objective of this work is to characterize the hyperelastic behavior of thermoplastic sheets used in
the process of thermoforming, blow molding or injection blow molding, with other modeling methods than
conventional methods, by exploiting the robustness of neuronal models.The results have accentuated the
strength of the model chosen to reproduce the behavior of membranes, regardless of material or geometric
nonlinearities presented in the study of such materials.A conclusion section must be included and should
indicate clearly the advantages, limitations, and possible applications of the paper. Although a conclusion may
review the main points of the paper, do not replicate the abstract as the conclusion. A conclusion might
elaborate on the importance of the work or suggest applications and extensions.
REFERENCES
[1] Rasmussen, H. K., J. H. Christensen and S. Gottsche, Inflation of polymer melts into elliptic and circular cylinders, J. Non-
Newtonian Fluid Mech. 93(2–3), 245–263, 2000
[2] Joye, D. D., Poehlein, G.W. and Denson, C. D. A Bubble Inflation Technique for the Measurement of Viscoelastic Properties in
Equal Biaxial Extension Flow, II Trans. Soc. Rheol., 16: 421–445, 1972
[3] J. Hopfield, Neural networks and physical systems with emergent collective computational abilities. Proceeding of the National
Academy of sciences of the United States of America, 1982
[4] P. Borne, M. Benrejeb, J. Haggège, Les réseaux de neurones : présentation et applications, Paris : Technip 2007
[5] F, Erchiquiet. A, Derdouri, Analyse Expérimentale et Numérique du Analyse Expérimentale et Numérique du Comportement de
Membranes Thermoplastiques en ABS et en HIPS dans le Procédé de Thermoformage, the canadian journal of chemical
engineering, vol 83, 2005
[6] W. McCulloch, W. Pitts, A Logical Calculus of the Ideas Immanent in Nervous Activity, Bulletin of Mathematical Biophysics, vol.
5, pp. 115-133, 1943
[7] Levenberg, K. A Method for the Solution of Certain Nonlinear Problems in Least Squares, Quarterly of Applied Mathematics, 2(2):
164–168, 1944
[8] Marquardt, D. An Algorithm for Least Squares Estimation of Nonlinear Parameters, SIAM Journal on Applied Mathematics, 11(2):
431–441, 1963
[9] P. Davis, Levenberg-Marquardt Methods and Nonlinear Estimation, SIAM News, Vol. 26, Number 6, 1993
[10] Ogden, R. W. Large Deformation Isotropic Elasticity – on the Correlation of Theory and Experiment for Incompressible Rubberlike
Solids, Proc. R. Soc. Lond., A326: 565–584, 1972
[11] F. Erchiqui, Analyse Expérimentale et Numérique du Comportement de Membranes Thermoplastiques en ABS et en HIPS dans le
Procédé de Thermoformage, the canadian journal of chemical engineering, Volume 83, 2005

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  • 1. Research Inventy: International Journal Of Engineering And Science Vol.2, Issue 8 (March 2013), Pp 18-22 Issn(e): 2278-4721, Issn(p):2319-6483, Www.Researchinventy.Com 18 Characterization of Polymeric Membranes under Large Deformations by a Neural Model Farid Hicham1,2 , El Ghorba Mohamed1 , Erchiqui Fouad2 , M’hamed Chergui1 1 Laboratoire de Contrôle et Caractérisation Mécanique des Matériaux et des Structures ENSEM, B.P 8118, Oasis-Route El Jadida Casablanca, Maroc 2 Laboratoire de Bioplasturgie et Nanotechnologie, UQAT, 445, boul. de l’Université, Rouyn-Noranda (QC), Canada J9X 5E4 Abstract: Recent progress in polymers modeling shows a need for a precise description of the material behavior under the combined effect of the applied efforts and temperature.The Artificial Neural Networks (ANN), whose operation is based on some properties of biological neurons, contain various architectures strongly interrelated treating elements and offering an alternative to conventional computational approaches. They respond in parallel to a set of inputs, and are affected by transformations more than by algorithms and procedures. They can achieve complicated operations of Input-Output without explicit relationships (linear and nonlinear) between all the presented data during a learning process.In our work, we are interested by the characterization of circular thermoplastic membranes, ABS (Acrylonitrile butadiene styrene), under biaxial deformation using the free blowing technique. Hyperelastic Mooney-Rivlin model is considered. A neural algorithm (based on artificial neural networks) is used to model the behavior of blowing these membranes, the results are compared with experimental studies and numerical finite differences model. Key words : membrane, Artificial Neural Networks, free blowing, hyperelasticity, ABS. I. INTRODUCTION Working a polymeric sheet attached by its contour in a 3D shape is the main feature of the process of blow molding. Generally, the deformation is very fast, non-uniform, multiaxial, and occurs at a forming temperature above the glass transition temperature [1]. The modeling of this phenomenon remains delicate and creates several difficulties as in the experimentation level [2] as in the modeling level in terms of important computational time, as well as the implementation of nonlinear constitutive laws... Often, as the bubble size increases and the internal pressure approach a maximum value beyond it there no solution, the numerical scheme diverges. So, to remedy this problem, we consider in this work, an approach based on an artificial neural networks model [3], to model the behavior of thermoplastic membranes. Recently, neural networks are used in many areas include the classification, pattern recognition, speech synthesis, diagnosis, identification and control of dynamic systems, or even to improve the quality of produced parts in various industrial processes such as injection molding or blow molding. The use of neural networks in the identification processes is justified by the fact that they can be well approximated nonlinear functions through their capacity to reproduce rather complex behavior, and their performances are improving so continuously while relying on a dynamic learning [4], which provides a robust neuronal identification vis-à-vis the parametric variations and disturbances that can affect the operation of the system studied. Modeling using neural networks requires among a model selection which is a crucial step in designing a neural network, as with any non-linear model. Indeed, this phase should lead to choose the model that has a complexity that is both sufficient to fit the data and not excessive.In this work, the power of neural networks is used to model the nonlinear behavior in free bowing of a polymeric membrane in ABS. A multilayer neural network is used for this application, in order to reproduce the behavior of this membrane; the results are compared with experimentation as well as with finite difference model [5]. II. ARTIFICIAL NEURAL NETWORKS 2.1 Introduction Neural networks have been studied since the 40's with the notion of formal neuron of McCulloch and Pitts [6] who first developed a mathematical model of biological neuron.Hence a neural network is a mathematical model of treatment consists of several basic interconnected neurons via weights that play the role
  • 2. Characterization Of Polymeric Membranes Under Large… 19 of synapses. These weights assume values that define the behavior of the whole structure. The adaptation of the latter through a suitable learning algorithm, allows the network to learn, memorize and generalize information. 2.2 Multilayer network 2.2 Architecture In general, a multilayer network is composed of an input layer, an output layer, and a number of hidden layers. Each neuron is connected to all neurons of the next layer via connections whose weights are real. Usually, the neuron used in the hidden layers or in the output layer, performs a weighted summation of its inputs and a nonlinear transformation which is often the sigmoid function. While the neuron used in the input layer, simply passes its input to output. The architecture of a multilayer network can be given by the following figure, Fig 1 : Figure 1. Architecture of a multilayer perceptron 2.3 Learning process The learning of a neural network means that it changes its behavior to allow it to move towards a clearly defined purpose. In other words, learning is adjusting the connection weights so that the outputs of the network are as close as possible to the desired outputs for all the used examples.Initially, the learning of multilayer networks was determined by the gradient method. Then, all optimization methods have been applied to this problem as the conjugate gradient method, the Levenberg-Marquardt [7,8]or Kalman filters… Thus, the literature on learning of multilayer neural networks is very rich. However, we limit the study of the back- propagation algorithm combined with a Levenberg-Marquardt optimization algorithm, which is a modified version of the gradient method and remains the most used and most responded. This is an optimization algorithm that seeks to minimize a cost function which covers the gap between the desired output and that delivered by the network, to expand more knowledge, we bring the reader to references [4] and [9]. The back-propagation algorithm can be described using the following two phases:Propagation phase or relaxation: initially, the input values are provided to the network’s input layer, then the network propagates the information from one layer to another to the output layer, and which gives the response of network. Back-propagation phase: that is to calculate the difference between the outputs of the network and the desired resulting changes in weight of the output neurons. Then, retro-propagating the error to the input layer which allows the adaptation of the weights of the hidden layer. In our network, we used a learning algorithm by back-propagation associated with a Levenberg-Marquardt optimization algorithm [9], with a transfer function of sigmoid type. In our architecture, the error in the presentation of an example, denoted by E, can be given by the following expression: (1) wherein, represents the component of the desired output vector. The overall error to minimize is the sum of all errors on the database. The inputs and outputs of the neurons j and k explicit from the following expressions: (2)
  • 3. Characterization Of Polymeric Membranes Under Large… 20 (3) Where f is the sigmoid activation function defined by: (4) The adjustment of the weights of the network by the back-propagation algorithm is ensured through the following iterative equation: (5) With ε and i denote the pitch and the iteration number. The derivative of E with the weight depends on its position, in fact: If the weight connects the hidden layer to the output layer, so: (6) If the weight connects the input layer to the hidden layer, then: (7) It should be emphasized that the convergence of the back-propagation algorithm depends on a variety of parameters, namely: The complexity of the database and the order of presentation of examples. Indeed, various studies have shown that a random sample presentation allows faster learning,The structure of the neural network considered and especially the number of neurons in the hidden layer which must not be very important to ensure the generalization ability of the network, or very small for the network to learn,The initial setting of the algorithm parameters, essentially the initial values of weight and iteration pitch must be chosen in a manner allowing to have a fast convergence. The multilayer neural network that we propose has the following structure: Figure 2. Structure of the used multilayer neural network The used network consists of an input layer, hidden layers, and an output layer. The number of neurons in the output layer depends on the response contemplated by the network. For the identification program, two neurons are required in the output layer to give the response of the excitation, while the input of the network is the variance of the corresponding pressures. As for modeling behavior of the membrane, the neuron will output variance in response to pressure, while the input will be presented by the stretch ratios.The experimental data are used for network learning, also, the back-propagation algorithm is used for error of perceptron learning. Thus, the optimization algorithm of Levenberg-Marquardt is used also in view of minimizing the error during the operation of back propagation, this optimization technique is more powerful than other optimization algorithms, but it requires more memory. Inputlayercontainingan excitationvector Multilayer neural networks Outputlayercontaininga responsevector
  • 4. Characterization Of Polymeric Membranes Under Large… 21 III. EXPERIMENTAL The materials considered in this work is the ABS (Acrylonitrile butadiene styrene). The initial sheet thickness was 0.46mm. The exposed circular domain of radius R=3.175 cm is heated to the softening point inside a heating chamber using infrared heaters. When the temperature was quite uniform over the flat sheet, the inflation was started using compressed air at a controlled flow rate. In most inflation tests the experiment ended when the bubble burst. The bubble pressure, its height at the pole and time are recorded simultaneously using a video camera and a data acquisition system. IV. RESULTS Fig 3 below shows a comparison between our neural model, finite difference model using a hyperelastic Ogden model [10, 11], and experimental measurements. Figure 3. Internal pressure versus the bubble height, comparison between experimental results, finite difference model, and neural networks model Note that the neural model we propose reproduces faithfully the behavior of the ABS membrane as well as the finite difference model. The margin of error between the neural model and the experimental curve remains negligible, and can also be minimized while depending on the choice of the number of hidden layers in the network and the chosen optimization algorithm. By increasing the number of hidden layers in the network, while keeping the same transfer function and the same optimization algorithm of Levenberg-Marquardt, the neuronal model can be adjusted for more fitting with the experimental results, Fig 4 below shows the results of model fitting: Figure 4. Internal pressure versus the bubble height, comparison between experimental results, finite difference model, and neural networks model (Adjusted model) It is clear that the neural model that we propose reproduces the behavior of the membrane, but, the fitting procedure that contains a number of algorithms, affects the computation time which becomes increasingly important also with increasing the number of hidden layers in the network, which induces the addition of other conditions nonlinearity.
  • 5. Characterization Of Polymeric Membranes Under Large… 22 V. CONCLUSION The objective of this work is to characterize the hyperelastic behavior of thermoplastic sheets used in the process of thermoforming, blow molding or injection blow molding, with other modeling methods than conventional methods, by exploiting the robustness of neuronal models.The results have accentuated the strength of the model chosen to reproduce the behavior of membranes, regardless of material or geometric nonlinearities presented in the study of such materials.A conclusion section must be included and should indicate clearly the advantages, limitations, and possible applications of the paper. Although a conclusion may review the main points of the paper, do not replicate the abstract as the conclusion. A conclusion might elaborate on the importance of the work or suggest applications and extensions. REFERENCES [1] Rasmussen, H. K., J. H. Christensen and S. Gottsche, Inflation of polymer melts into elliptic and circular cylinders, J. Non- Newtonian Fluid Mech. 93(2–3), 245–263, 2000 [2] Joye, D. D., Poehlein, G.W. and Denson, C. D. A Bubble Inflation Technique for the Measurement of Viscoelastic Properties in Equal Biaxial Extension Flow, II Trans. Soc. Rheol., 16: 421–445, 1972 [3] J. Hopfield, Neural networks and physical systems with emergent collective computational abilities. Proceeding of the National Academy of sciences of the United States of America, 1982 [4] P. Borne, M. Benrejeb, J. Haggège, Les réseaux de neurones : présentation et applications, Paris : Technip 2007 [5] F, Erchiquiet. A, Derdouri, Analyse Expérimentale et Numérique du Analyse Expérimentale et Numérique du Comportement de Membranes Thermoplastiques en ABS et en HIPS dans le Procédé de Thermoformage, the canadian journal of chemical engineering, vol 83, 2005 [6] W. McCulloch, W. Pitts, A Logical Calculus of the Ideas Immanent in Nervous Activity, Bulletin of Mathematical Biophysics, vol. 5, pp. 115-133, 1943 [7] Levenberg, K. A Method for the Solution of Certain Nonlinear Problems in Least Squares, Quarterly of Applied Mathematics, 2(2): 164–168, 1944 [8] Marquardt, D. An Algorithm for Least Squares Estimation of Nonlinear Parameters, SIAM Journal on Applied Mathematics, 11(2): 431–441, 1963 [9] P. Davis, Levenberg-Marquardt Methods and Nonlinear Estimation, SIAM News, Vol. 26, Number 6, 1993 [10] Ogden, R. W. Large Deformation Isotropic Elasticity – on the Correlation of Theory and Experiment for Incompressible Rubberlike Solids, Proc. R. Soc. Lond., A326: 565–584, 1972 [11] F. Erchiqui, Analyse Expérimentale et Numérique du Comportement de Membranes Thermoplastiques en ABS et en HIPS dans le Procédé de Thermoformage, the canadian journal of chemical engineering, Volume 83, 2005