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Radiation Measurements 43 (2008) 332–334
www.elsevier.com/locate/radmeas
Application of the OSL technique for beta dosimetry
T.N.O. Pintoa,b
, S.G.P. Cecattia,b,∗
, C.C. Gronchia,b
, L.V.E. Caldasb
aFundacentro, Ministério do Trabalho e Emprego, São Paulo, SP, Brazil
bInstituto de Pesquisas Energéticas e Nucleares, Comissão Nacional de Energia Nuclear, São Paulo, SP, Brazil
Abstract
In recent years, the optically stimulated luminescence (OSL) technique has been used in personal dosimetry, and aluminum oxide (Al2O3:C)
has become a very useful material for this technique. The objective of this work is to study the dosimetric characterization of Al2O3:C for beta
radiation detection using the OSL method. The results obtained show that for monitoring of workers exposed to beta radiation, the technique
and the material are useful, but the energy dependence of the OSL response of Al2O3:C has to be taken into consideration.
© 2007 Elsevier Ltd. All rights reserved.
Keywords: Optically stimulated luminescence; Beta radiation; Al2O3:C
1. Introduction
When workers handle radioactive materials they may expose
their extremities to doses significantly greater than the whole
body dose. Beta radiation may cause damage to the workers in
these cases, and then extremity dosimeters become extremely
important (Durhan et al., 2002).
The main requirement of a personal dosimeter for the moni-
toring of beta radiation doses is the capability of measuring the
ICRU quantity of Hp (0.07) with satisfactory accuracy, inde-
pendently of the radiation incident angle and the beta radiation
energy (Akselrod et al., 1999).
Beta dosimetry presents more difficulties than gamma
dosimetry, since skin dose is defined at a single depth in tissue,
and the dose deposition from beta particles in tissue is highly
non-uniform. Dosimeters with a finite thickness yield the dose
averaged over the thickness of the dosimeter (Durham et al.,
2002).
In extremity dosimetry the dose should preferably be mea-
sured using a very thin dosimeter, particularly for beta dosime-
try (Akselrod et al., 1996). Extremity dosimeters have to be
produced in very thin layers with sufficient sensitivity to pro-
vide accurate dose measurements between 1 mGy and 10 Gy.
∗ Corresponding author. Fundacentro, Ministério do Trabalho e Emprego,
São Paulo, SP, Brazil. Tel.: +55 11 30666210; fax: +55 11 3816 9117.
E-mail address: scecatti@fundacentro.gov.br (S.G.P. Cecatti).
1350-4487/$ - see front matter © 2007 Elsevier Ltd. All rights reserved.
doi:10.1016/j.radmeas.2007.10.024
Various types of thin detectors have been prepared and tested
using highly sensitive thermoluminescent (TL) phosphors, e.g.
MgB4O7:Dy; CaSO4:Dy; Al2O3:C and LiF:Mg,Cu,P (Campos
and Lima, 1987); (Akselrod et al., 1996).
Aluminum oxide (Al2O3:C) was initially developed as a
TL material. In recent years, the optically stimulated lumines-
cence (OSL) technique has been used in personal dosimetry,
and Al2O3:C has become a material of choice for this technique
(Akselrod et al., 1999).
The Al2O3:C detectors present very good dosimetric prop-
erties, and they have become successful personal OSL dosime-
ters (Akselrod et al., 1990; McKeever et al., 1996; McKeever,
2001). Thin layers of this material can be used to measure dif-
ferent energies of beta radiation, within the limits established
in the US by the National Voluntary Laboratory Accreditation
Program and the US Department of Energy Laboratory Ac-
creditation Program with acceptable accuracy (Akselrod et al.,
1999).
The objective of this work is the dosimetric characterization
of Al2O3:C for beta radiation detection using the OSL method
in order to monitor workers exposed to beta radiation.
2. Materials and methods
The beta irradiations of the OSL detectors were performed
using the beta secondary standard system of the Calibration
Laboratory at IPEN, with 90Sr +90Y, 85Kr and 147Pm sources,
T.N.O. Pinto et al. / Radiation Measurements 43 (2008) 332–334 333
Table 1
Characteristics of the secondary standard system of beta radiation
Source 147Pm 85Kr 90Sr + 90Y
Nominal activity (MBq) 3700 3700 460
Mean beta energy (MeV) 0.06 0.69 0.80
Absorbed dose rate in
air ( Gy s−1)
2.35 ± 0.05 39.7 ± 0.5 16.46 ± 0.22
Calibration distance (cm) 20 30 30
Reference date 19/11/2004 30/11/2004 08/12/2004
manufactured by AEA Technology, Germany, and calibrated
by the primary standard laboratory, Physikalisch - Technische
Bundesanstalt (PTB), Germany. The radiation source charac-
teristics can be seen in Table 1.
The measurements were obtained using OSL dot dosimeters
of Al2O3:C with a Landauer microStar reader and software.
This detector is a layer of Al2O3:C sandwiched between two
layers of polyester for a total thickness of 0.3 mm and diameter
of 0.7 mm (Landauer, 2006).
For the irradiations, each OSL dot dosimeter of Al2O3:C
was positioned on a polymethylmethacrylate (PMMA) phantom
(120 mm × 120 mm × 15 mm). The dots were irradiated at
the phantom surface–source distance of 30 cm in the cases of
90Sr+90Y and 85Kr, and at 20 cm in the case of 147Pm, because
the absorbed dose rates were determined at those distances by
the PTB laboratory.
The measurements were always taken immediately after irra-
diation. The detectors were optically treated at 26×103
lux for
1 h prior to being re-utilized. A Delta OHM radiometer, model
D09721, LUX LP 9021PHOT sensor, was utilized to determine
the light level. (Gronchi et al., 2007).
3. Results
3.1. Reproducibility
The reproducibility of the OSL response of Al2O3:C detec-
tors was obtained by taking 10 measurements of each OSL
dosimeter, irradiated with an absorbed dose of 0.6 mGy of beta
radiation (90Sr + 90Y). The reproducibility obtained of the
Al2O3:C detectors was 2.5% (1 ).
3.2. Dose–response curve
The OSL dots of Al2O3:C were irradiated with 90Sr +90Y in
the dose range of 0.1–10 mGy. Ten dots were utilized for each
dose level. The dose–response curve presents (Fig. 1) a linear
response for low doses, which are more probable to occur in
occupational dosimetry. The error bars correspond to 1 .
3.3. Energy dependence
The OSL dot dosimeters were exposed to a dose of 3 mGy of
beta radiation of 90Sr +90Y and 85Kr, and to a dose of 13 mGy
of 147Pm. The results were normalized to the 90Sr +90Y mean
10-2
10-1
100
101
102
10-2
10-1
100
101
102
OSLResponse(a.u.)
Absorbed Dose (mGy)
90
Sr + 90
Y
Fig. 1. Dose–response curve of OSL response of Al2O3:C dot dosimeters to
beta radiation (90Sr + 90Y).
10-2
10-1
100
101
10-2
10-1
100
101
OSLResponse(a.u.)
Energy (MeV)
90
Sr + 90
Y
85
Kr
147
Pm
Fig. 2. Energy dependence of OSL response of Al2O3:C dot dosimeters to
beta radiation.
energy and divided by the absorbed doses (Fig. 2). Due to the
low radiation energy, in the case of the 147Pm source, the ab-
sorbed dose rate had to be corrected for the environmental stan-
dard conditions of 20 ◦C, 101.3 kPa and 50% relative humidity.
The curve was obtained using the Origin software “spline”
curve correction to link the three main points. The response
is given per unit dose and error bars are 1 . These materials
present a very high dependence of the OSL response on the
334 T.N.O. Pinto et al. / Radiation Measurements 43 (2008) 332–334
beta radiation energy, which has to be taken into consideration
for beta monitoring. The energy dependence curve obtained
for the Al2O3:C pellets irradiated with different beta sources
is comparable to that presented by Akselrod et al. (1999). The
energy response for beta radiation can be flatted by using filters
as discussed by Akselrod et al. (1996).
4. Conclusion
Al2O3:C dot dosimeters were characterized for beta radia-
tion dosimetry using the OSL technique in this work. The re-
producibility of OSL response was 2.5%.
The dose–response curve presents a linear response in the
low dose range of 0.1–10 mGy; these doses are more probable
to occur in occupational dosimetry.
The material presents a high energy dependence that has to
be taken into consideration for beta occupational dosimetry.
As discussed by Akselrod et al. (1996), filters may be used to
flatten this energy dependence curve.
The results on the main dosimetric characteristics investi-
gated in this paper show that the OSL dot dosimeters may be
useful for extremity dosimetry of workers exposed to beta ra-
diation, taking the energy dependence into consideration.
Acknowledgments
The authors are very grateful to Fundação de Amparo à
Pesquisa do Estado de São Paulo (FAPESP) and to Con-
selho Nacional de Desenvolvimento Científico e Tecnológico
(CNPq), Brazil, for partial financial support.
References
Akselrod, M.S., Kortov, V.S., 1990. Thermoluminescent and exoemission
properties of new high-sensitivity TLD -Al2O3:C crystals. Radiat. Prot.
Dosimetry 33, 123–126.
Akselrod, M.S., McKeever, S.W.S., Moscovitch, M., Emfietzoglou, D.,
Durham, J.S., Soares, C.G., 1996. A thin-layer Al2O3 beta TL detector.
Radiat. Prot. Dosimetry 66, 105–110.
Akselrod, A., Akselrod, M.S., Larsen, N.A., Banerjee, D., Botter-Jensen, L.,
Christensen, P., Lucas, A.C., McKeever, S.W.S., Yoder, R.C., 1999. Optical
stimulated luminescence response of Al2O3 to beta radiation. Radiat. Prot.
Dosimetry 85, 125–128.
Campos, L.L., Lima, M.F., 1987. Thermoluminescent CaSO4:Dy Teflon
pellets for beta radiation detection. Radiat. Prot. Dosimetry 18, 95–97.
Durham, J.S., Zhang, X., Payne, F., Akselrod, M.S., 2002. Design of a finger
ring extremity dosemeter based on OSL readout of alpha-Al2O3:C. Radiat.
Prot. Dosimetry 101, 65–68.
Gronchi, C.C., Cecatti, S.G.P., Pinto, T.C.N.O., Caldas, L.V.E., 2007. Light
induced fading of the OSL response of Al2O3:C detectors. In: Proceedings
of the International Nuclear Atlantic Conference, September 29–October
5, Santos, Brazil.
Landauer, 2006. User manual InLigth Systems. Laudauer, Illinois.
McKeever, S.W.S., 2001. Optically stimulated luminescence dosimetry. Nucl.
Instrum. and Methods Phys. Res. B 184, 29–54.
McKeever, S.W.S., Akselrod, M.S., Markey, B.G., 1996. Pulsed optically
stimulated dosimetry using -Al2O3. Radiat. Prot. Dosimetry 65,
267–272.

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Application of-the-osl-technique-for-beta-dosimetry 2008-radiation-measurements

  • 1. Radiation Measurements 43 (2008) 332–334 www.elsevier.com/locate/radmeas Application of the OSL technique for beta dosimetry T.N.O. Pintoa,b , S.G.P. Cecattia,b,∗ , C.C. Gronchia,b , L.V.E. Caldasb aFundacentro, Ministério do Trabalho e Emprego, São Paulo, SP, Brazil bInstituto de Pesquisas Energéticas e Nucleares, Comissão Nacional de Energia Nuclear, São Paulo, SP, Brazil Abstract In recent years, the optically stimulated luminescence (OSL) technique has been used in personal dosimetry, and aluminum oxide (Al2O3:C) has become a very useful material for this technique. The objective of this work is to study the dosimetric characterization of Al2O3:C for beta radiation detection using the OSL method. The results obtained show that for monitoring of workers exposed to beta radiation, the technique and the material are useful, but the energy dependence of the OSL response of Al2O3:C has to be taken into consideration. © 2007 Elsevier Ltd. All rights reserved. Keywords: Optically stimulated luminescence; Beta radiation; Al2O3:C 1. Introduction When workers handle radioactive materials they may expose their extremities to doses significantly greater than the whole body dose. Beta radiation may cause damage to the workers in these cases, and then extremity dosimeters become extremely important (Durhan et al., 2002). The main requirement of a personal dosimeter for the moni- toring of beta radiation doses is the capability of measuring the ICRU quantity of Hp (0.07) with satisfactory accuracy, inde- pendently of the radiation incident angle and the beta radiation energy (Akselrod et al., 1999). Beta dosimetry presents more difficulties than gamma dosimetry, since skin dose is defined at a single depth in tissue, and the dose deposition from beta particles in tissue is highly non-uniform. Dosimeters with a finite thickness yield the dose averaged over the thickness of the dosimeter (Durham et al., 2002). In extremity dosimetry the dose should preferably be mea- sured using a very thin dosimeter, particularly for beta dosime- try (Akselrod et al., 1996). Extremity dosimeters have to be produced in very thin layers with sufficient sensitivity to pro- vide accurate dose measurements between 1 mGy and 10 Gy. ∗ Corresponding author. Fundacentro, Ministério do Trabalho e Emprego, São Paulo, SP, Brazil. Tel.: +55 11 30666210; fax: +55 11 3816 9117. E-mail address: scecatti@fundacentro.gov.br (S.G.P. Cecatti). 1350-4487/$ - see front matter © 2007 Elsevier Ltd. All rights reserved. doi:10.1016/j.radmeas.2007.10.024 Various types of thin detectors have been prepared and tested using highly sensitive thermoluminescent (TL) phosphors, e.g. MgB4O7:Dy; CaSO4:Dy; Al2O3:C and LiF:Mg,Cu,P (Campos and Lima, 1987); (Akselrod et al., 1996). Aluminum oxide (Al2O3:C) was initially developed as a TL material. In recent years, the optically stimulated lumines- cence (OSL) technique has been used in personal dosimetry, and Al2O3:C has become a material of choice for this technique (Akselrod et al., 1999). The Al2O3:C detectors present very good dosimetric prop- erties, and they have become successful personal OSL dosime- ters (Akselrod et al., 1990; McKeever et al., 1996; McKeever, 2001). Thin layers of this material can be used to measure dif- ferent energies of beta radiation, within the limits established in the US by the National Voluntary Laboratory Accreditation Program and the US Department of Energy Laboratory Ac- creditation Program with acceptable accuracy (Akselrod et al., 1999). The objective of this work is the dosimetric characterization of Al2O3:C for beta radiation detection using the OSL method in order to monitor workers exposed to beta radiation. 2. Materials and methods The beta irradiations of the OSL detectors were performed using the beta secondary standard system of the Calibration Laboratory at IPEN, with 90Sr +90Y, 85Kr and 147Pm sources,
  • 2. T.N.O. Pinto et al. / Radiation Measurements 43 (2008) 332–334 333 Table 1 Characteristics of the secondary standard system of beta radiation Source 147Pm 85Kr 90Sr + 90Y Nominal activity (MBq) 3700 3700 460 Mean beta energy (MeV) 0.06 0.69 0.80 Absorbed dose rate in air ( Gy s−1) 2.35 ± 0.05 39.7 ± 0.5 16.46 ± 0.22 Calibration distance (cm) 20 30 30 Reference date 19/11/2004 30/11/2004 08/12/2004 manufactured by AEA Technology, Germany, and calibrated by the primary standard laboratory, Physikalisch - Technische Bundesanstalt (PTB), Germany. The radiation source charac- teristics can be seen in Table 1. The measurements were obtained using OSL dot dosimeters of Al2O3:C with a Landauer microStar reader and software. This detector is a layer of Al2O3:C sandwiched between two layers of polyester for a total thickness of 0.3 mm and diameter of 0.7 mm (Landauer, 2006). For the irradiations, each OSL dot dosimeter of Al2O3:C was positioned on a polymethylmethacrylate (PMMA) phantom (120 mm × 120 mm × 15 mm). The dots were irradiated at the phantom surface–source distance of 30 cm in the cases of 90Sr+90Y and 85Kr, and at 20 cm in the case of 147Pm, because the absorbed dose rates were determined at those distances by the PTB laboratory. The measurements were always taken immediately after irra- diation. The detectors were optically treated at 26×103 lux for 1 h prior to being re-utilized. A Delta OHM radiometer, model D09721, LUX LP 9021PHOT sensor, was utilized to determine the light level. (Gronchi et al., 2007). 3. Results 3.1. Reproducibility The reproducibility of the OSL response of Al2O3:C detec- tors was obtained by taking 10 measurements of each OSL dosimeter, irradiated with an absorbed dose of 0.6 mGy of beta radiation (90Sr + 90Y). The reproducibility obtained of the Al2O3:C detectors was 2.5% (1 ). 3.2. Dose–response curve The OSL dots of Al2O3:C were irradiated with 90Sr +90Y in the dose range of 0.1–10 mGy. Ten dots were utilized for each dose level. The dose–response curve presents (Fig. 1) a linear response for low doses, which are more probable to occur in occupational dosimetry. The error bars correspond to 1 . 3.3. Energy dependence The OSL dot dosimeters were exposed to a dose of 3 mGy of beta radiation of 90Sr +90Y and 85Kr, and to a dose of 13 mGy of 147Pm. The results were normalized to the 90Sr +90Y mean 10-2 10-1 100 101 102 10-2 10-1 100 101 102 OSLResponse(a.u.) Absorbed Dose (mGy) 90 Sr + 90 Y Fig. 1. Dose–response curve of OSL response of Al2O3:C dot dosimeters to beta radiation (90Sr + 90Y). 10-2 10-1 100 101 10-2 10-1 100 101 OSLResponse(a.u.) Energy (MeV) 90 Sr + 90 Y 85 Kr 147 Pm Fig. 2. Energy dependence of OSL response of Al2O3:C dot dosimeters to beta radiation. energy and divided by the absorbed doses (Fig. 2). Due to the low radiation energy, in the case of the 147Pm source, the ab- sorbed dose rate had to be corrected for the environmental stan- dard conditions of 20 ◦C, 101.3 kPa and 50% relative humidity. The curve was obtained using the Origin software “spline” curve correction to link the three main points. The response is given per unit dose and error bars are 1 . These materials present a very high dependence of the OSL response on the
  • 3. 334 T.N.O. Pinto et al. / Radiation Measurements 43 (2008) 332–334 beta radiation energy, which has to be taken into consideration for beta monitoring. The energy dependence curve obtained for the Al2O3:C pellets irradiated with different beta sources is comparable to that presented by Akselrod et al. (1999). The energy response for beta radiation can be flatted by using filters as discussed by Akselrod et al. (1996). 4. Conclusion Al2O3:C dot dosimeters were characterized for beta radia- tion dosimetry using the OSL technique in this work. The re- producibility of OSL response was 2.5%. The dose–response curve presents a linear response in the low dose range of 0.1–10 mGy; these doses are more probable to occur in occupational dosimetry. The material presents a high energy dependence that has to be taken into consideration for beta occupational dosimetry. As discussed by Akselrod et al. (1996), filters may be used to flatten this energy dependence curve. The results on the main dosimetric characteristics investi- gated in this paper show that the OSL dot dosimeters may be useful for extremity dosimetry of workers exposed to beta ra- diation, taking the energy dependence into consideration. Acknowledgments The authors are very grateful to Fundação de Amparo à Pesquisa do Estado de São Paulo (FAPESP) and to Con- selho Nacional de Desenvolvimento Científico e Tecnológico (CNPq), Brazil, for partial financial support. References Akselrod, M.S., Kortov, V.S., 1990. Thermoluminescent and exoemission properties of new high-sensitivity TLD -Al2O3:C crystals. Radiat. Prot. Dosimetry 33, 123–126. Akselrod, M.S., McKeever, S.W.S., Moscovitch, M., Emfietzoglou, D., Durham, J.S., Soares, C.G., 1996. A thin-layer Al2O3 beta TL detector. Radiat. Prot. Dosimetry 66, 105–110. Akselrod, A., Akselrod, M.S., Larsen, N.A., Banerjee, D., Botter-Jensen, L., Christensen, P., Lucas, A.C., McKeever, S.W.S., Yoder, R.C., 1999. Optical stimulated luminescence response of Al2O3 to beta radiation. Radiat. Prot. Dosimetry 85, 125–128. Campos, L.L., Lima, M.F., 1987. Thermoluminescent CaSO4:Dy Teflon pellets for beta radiation detection. Radiat. Prot. Dosimetry 18, 95–97. Durham, J.S., Zhang, X., Payne, F., Akselrod, M.S., 2002. Design of a finger ring extremity dosemeter based on OSL readout of alpha-Al2O3:C. Radiat. Prot. Dosimetry 101, 65–68. Gronchi, C.C., Cecatti, S.G.P., Pinto, T.C.N.O., Caldas, L.V.E., 2007. Light induced fading of the OSL response of Al2O3:C detectors. In: Proceedings of the International Nuclear Atlantic Conference, September 29–October 5, Santos, Brazil. Landauer, 2006. User manual InLigth Systems. Laudauer, Illinois. McKeever, S.W.S., 2001. Optically stimulated luminescence dosimetry. Nucl. Instrum. and Methods Phys. Res. B 184, 29–54. McKeever, S.W.S., Akselrod, M.S., Markey, B.G., 1996. Pulsed optically stimulated dosimetry using -Al2O3. Radiat. Prot. Dosimetry 65, 267–272.